Abstract
Point-of-use treatment technologies can increase access to safe drinking water in rural areas. Sustained use of these technologies is uncommon due to oversight of community needs, user-perceived risks, long-term maintenance, and conflict with traditional practices. Nanosilver-enabled ceramic water filters are unique due to the use of locally sourced materials available at or near the target community; however, technical limitations persist (e.g., nanosilver’s uncontrolled release and passivation from sulfide or chloride). This work aims to overcome these limitations by impregnating nanosilver onto ceramics with a Navajo pottery rosin, collected from pinyon trees with a third-generation artisan. Here, we investigate this sustainable and novel material for drinking water treatment; the study ranges from a proof of concept to testing under realistic conditions. Results show that when embedded in a thin film, the biopolymer controlled ionic silver dissolution and prevented silver passivation from sulfide and chloride. When applied to ceramic filters, the biopolymer effectively immobilized nanosilver in a range of waters. Over a 25 day study to emulate household-use conditions, this coating method sustained disinfection of a coculture of Gram-positive and Gram-negative bacteria while controlling biofouling. Overall, the use of this Navajo pottery material can facilitate adoption while providing the needed technological advancement to these widely used treatment devices.
| Original language | English |
|---|---|
| Pages (from-to) | 17132-17143 |
| Number of pages | 12 |
| Journal | Environmental Science and Technology |
| Volume | 57 |
| Issue number | 44 |
| DOIs | |
| State | Published - Oct 23 2023 |
Keywords
- Anti-Bacterial Agents
- Biopolymers
- Ceramics
- Chlorides
- Disinfection/methods
- Drinking Water
- Filtration/methods
- Gram-Negative Bacteria
- Gram-Positive Bacteria
- Metal Nanoparticles
- Silver
- Sulfides
- Water Purification/methods