TY - JOUR
T1 - Population trapping in short-pulse multiphoton ionization
AU - Edwards, Mark
AU - Clark, Charles W.
PY - 1996/1
Y1 - 1996/1
N2 - We have studied population trapping in a one-dimensional model atom interacting with a short-pulse high-intensity laser, using Floquet analysis and direct numerical integration of the time-dependent Schrödinger equation for a range of peak pulse intensities. We find that photoelectrons are efficiently produced only by pulses whose peak intensities lie in a narrow range around the resonant intensity for a given intermediate state. Excited-state populations, however, are generated with comparable efficiencies for all pulses whose peak intensities exceed the resonant intensity. This implies that, for a realistic laser pulse with an inhomogeneous spatial distribution of intensity, excited atoms are generated throughout a larger volume than are photoelectrons. Interpretations of recent experiments are reexamined in light of this result.
AB - We have studied population trapping in a one-dimensional model atom interacting with a short-pulse high-intensity laser, using Floquet analysis and direct numerical integration of the time-dependent Schrödinger equation for a range of peak pulse intensities. We find that photoelectrons are efficiently produced only by pulses whose peak intensities lie in a narrow range around the resonant intensity for a given intermediate state. Excited-state populations, however, are generated with comparable efficiencies for all pulses whose peak intensities exceed the resonant intensity. This implies that, for a realistic laser pulse with an inhomogeneous spatial distribution of intensity, excited atoms are generated throughout a larger volume than are photoelectrons. Interpretations of recent experiments are reexamined in light of this result.
UR - http://www.scopus.com/inward/record.url?scp=0030532697&partnerID=8YFLogxK
U2 - 10.1364/JOSAB.13.000101
DO - 10.1364/JOSAB.13.000101
M3 - Article
SN - 0740-3224
VL - 13
SP - 101
EP - 112
JO - Journal of the Optical Society of America B: Optical Physics
JF - Journal of the Optical Society of America B: Optical Physics
IS - 1
ER -