Population trapping in short-pulse multiphoton ionization

Mark Edwards, Charles W. Clark

Research output: Contribution to journalArticlepeer-review

8 Scopus citations

Abstract

We have studied population trapping in a one-dimensional model atom interacting with a short-pulse high-intensity laser, using Floquet analysis and direct numerical integration of the time-dependent Schrödinger equation for a range of peak pulse intensities. We find that photoelectrons are efficiently produced only by pulses whose peak intensities lie in a narrow range around the resonant intensity for a given intermediate state. Excited-state populations, however, are generated with comparable efficiencies for all pulses whose peak intensities exceed the resonant intensity. This implies that, for a realistic laser pulse with an inhomogeneous spatial distribution of intensity, excited atoms are generated throughout a larger volume than are photoelectrons. Interpretations of recent experiments are reexamined in light of this result.

Original languageEnglish
Pages (from-to)101-112
Number of pages12
JournalJournal of the Optical Society of America B: Optical Physics
Volume13
Issue number1
DOIs
StatePublished - Jan 1996

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